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As a first step toward development of novel inhibitors of Photosystem II (PS II) for controlling excess atmospheric CO2, a 2-fluorobenzoic acid ester was synthesized and characterized by X-ray crystallography. The phenol moiety was selected based on the phenol electron acceptor and the use of a 2-fluorophenyl moiety was adopted because only this group could react with the catalytic Mn ion, which is essential for the catalytic cycle of the water-splitting reaction. The X-ray structure revealed that the methoxy group of the ester could interact with residues close to the Mn ion, particularly with Arg190 and Glu176. These residues play an important role in the catalytic cycle of water splitting. Then, we tested the inhibitory activity of this compound toward PS II. A low-level of inhibition was observed in a 50-μM treatment with reduced oxygen evolution, although no photocatalytic activity of PS II was observed under these conditions. However, 1 and 10 μM treatments with intact oxygen evolution caused inhibition of PS II, particularly as judged by electrochemical analysis, which is consistent with the inhibitory effect of the ester. It is well known that PS II is the center of photoinhibition with overproduction of reactive oxygen species. The results indicate that the ester functions as an inhibitor for c-type cytochrome production in the electron transfer from plastoquinone to oxygen in PS II.Swimming at the 2011 Pan American Games – Men’s 200 metre freestyle

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A chronicle of an epic soccer journey that spans the globe. Eventually it reached the hands of once brother, Beckett. Siva. (born September 6, 1969), is an entrepreneur and the founder of

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